Built-in elastic strain and localization effects on GaAs luminescence of MOVPE-grown GaAs-AlGaAs core-shell nanowires

Abstract

The core photoluminescence emission of MOVPE-grown GaAs-Al0.33Ga0.67As core-shell nanowires is studied as function of the relevant geometrical parameter of these nanostructures, namely the shell-thickness to core-radius ratio hs/Rc. The energy of the dominant emission peak was compared with values of the GaAs heavy- and light-hole excitons redshifted by a uniaxial tensile strain, the latter calculated assuming perfect coherence at the core/shell interface and elastic energy equilibrium within the nanowires. Good agreement is obtained for hs/Rc < 1, the intrinsic strain-free excitonic emission being identified at 1.510 eV, and further ascribed to bound heavy-hole excitons. For hs/Rc > 1 increasingly larger redshifts (up to ∼9 meV in excess of values calculated based on our elastic strain model) are observed, and tentatively ascribed to shell-dependent exciton localization effects. Experimental and calculated bound exciton peak energies for GaAs-Al0.33Ga0.67As core-shell nanowires as function of their shell-thickness to core-radius ratio hs/Rc.


Autore Pugliese

Tutti gli autori

  • P. Prete , I. Miccoli , F. Marzo , N. LOVERGINE

Titolo volume/Rivista

PHYSICA STATUS SOLIDI. RAPID RESEARCH LETTERS


Anno di pubblicazione

2013

ISSN

1862-6254

ISBN

Non Disponibile


Numero di citazioni Wos

Nessuna citazione

Ultimo Aggiornamento Citazioni

Non Disponibile


Numero di citazioni Scopus

3

Ultimo Aggiornamento Citazioni

28/04/2018


Settori ERC

Non Disponibile

Codici ASJC

Non Disponibile